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2013-11-20
X-ray time delays in the Narrow Line Seyfert 1 galaxy PG 1244+026
We analyse the X-ray time-lags in the Narrow Line Seyfert 1 (NLS1) galaxy PG 1244+026 ($M_{\rm BH}\sim 10^7 M_{\rm sun}$, $L/L_{\rm Edd}\sim 1$). The time delay between the soft (0.3--0.7~keV) and harder (1.2--4.0~keV) variations shows shows the well established switch from hard lags at low frequencies to soft lags at high frequencies. The low frequency hard lags are qualitatively consistent with the propagation of fluctuations model, with some long-timescale response of the reflection component. The high frequency soft lag appears to extend over a wide frequency band, that we divide this into two narrow frequency ranges, and examine the lag as a function of energy for each of these. At high frequencies the soft excess emission is delayed with respect to the harder energy bands, without any corresponding strong, hard X-ray reflection signature. At even higher frequencies a soft lag is seen at the softest energies, as well as tentative evidence for an iron K$\alpha$ reverberation signal. These results point to the importance of reprocessing as well as reflection in determining the lags in NLS1s.
1311.5165v2
2013-11-21
L4Fe2As2Te1-xO4-yFy (L = Pr, Sm, Gd): a layered oxypnictide superconductor with Tc up to 45 K
The synthesis, structural and physical properties of iron lanthanide oxypnictide superconductors, L4Fe2As2Te1-xO4 (L = Pr, Sm, Gd), with transition temperature at ~ 25 K are reported. Single crystals have been grown at high pressure using cubic anvil technique. The crystal structure consists of layers of L2O2 tetrahedra separated by alternating layers of chains of Te and of Fe2As2 tetrahedra: -L2O2-Te-L2O2-Fe2As2-L2O2-Te-L2O2- (space group: I4/mmm, a ~ 4.0, c ~ 29.6 {\AA}). Substitution of oxygen by fluorine increases the critical temperature, e.g. in Gd4Fe2As2Te1-xOyF4-y up to 45 K. Magnetic torque measurements reveal an anisotropy of the penetration depths of ~31.
1311.5437v2
2013-11-22
Magnetic phase transitions and superconductivity in strained FeTe
The influence of hydrostatic pressure and ab-plane strain on the magnetic structure of FeTe is investigated from first principles. The results of calculations reveal a phase transition from antiferromagnetic double-stripe ordering at ambient pressure to ferromagnetic ordering at 2 GPa, or under compressive strain reducing the lattice parameter a by about 3%. In turn, a tensile strain of less than 2% induces the phase transition to antiferromagnetic single-stripe ordering. It corresponds to the superconducting FeTe thin films, thereby confirming that the superconducting state is positively linked to single-stripe antiferromagnetic fluctuations. Both types of transition indicate that the position of Te atoms in the crystal is crucial for the magnetic and superconducting properties of iron chalcogenides.
1311.5732v1
2013-11-22
Coherent emission of $γ$ quanta by synchrotron radiation excited nuclei: geometry of nearly backward scattering
A possibility of further development of Synchrotron M\"{o}ssbauer Source (SMS) of $^{57}$Fe 14.4 keV radiation is considered. The principles and detailed description of the SMS device is given in Refs. Phys. Rev. A 84, 053851 (2011) G. V. Smirnov et al, J. Synchrotron Rad., v. 19, 559 (2012) V. Potapkin et al. The perfect crystal of Iron Borate, FeBO$_{3}$, is the central element of this device. The coherent nuclear fluorescence of IB crystal illuminated by synchrotron radiation produces the sharply directed beam of 14.4 keV M\"{o}ssbauer radiation from the crystal set at the pure nuclear Bragg reflection. Up to now the low angle scattering geometry was used for generation of the coherent $\gamma $ radiation. The analysis performed in the present paper shows that the source of about two times larger power can be obtained when nearly backward scattering geometry is employed. This result can be efficiently applied in development of high resolution spectroscopy using synchrotron radiation.
1311.5771v1
2013-11-24
Temperature and high strain rate dependence of tensile deformation behavior in single crystal iron from dislocation dynamics simulations
We conduct dislocation dynamics (DD) simulations of Fe periodic single crystals under tensile load at several high strain rates and temperatures. The simulations are enabled by the recent development of temperature-dependent dislocation mobility relations obtained from atomistic calculations. The plastic evolution in the simulations is governed by rapid initial dislocation multiplication, followed by a saturation of the flow stress when the subpopulation of slow plastic carriers becomes stabilized by dislocation annihilation. Above 500 K, edge dislocations coexist with screw dislocations and contribute proportionaly to the value of the flow stress. The DD simulations are used to interpret shock-loading experiments in Fe in terms of the relative importance of different strengthening mechanisms. We find that in the $10^4$-to-$10^6$ s$^{-1}$ strain rate regime, work hardening explains the hardening of shock-loaded bulk Fe crystals.
1311.6173v1
2013-11-26
Field Measurement for Superconducting Magnets of ADS Injector I
The superconducting solenoid magnet prototype for ADS injection-I had been fabricated in Beijing Qihuan Mechanical and Electric Engineer Company and tested in Haerbin Institute of Technology (HIT) in Nov, 2012. Batch magnet production was processed after some major revision from the magnet prototype, they include: removing off the perm-alloy shield, extending the iron yoke, using thin superconducting cable, etc. The first one of the batch magnets was tested in the vertical Dewar in HIT in Sept. 2013. Field measurement was carried out at the same time by the measurement platform that seated on the top of the vertical Dewar. This paper will present the field measurement system design, measurement results and discussion on the residual field from the persistent current effect.
1311.6596v1
2013-11-28
From supernovae to neutron stars
The gravitational collapse, bounce, the explosion of an iron core of an 11.2 $M_{\odot}$ star is simulated by two-dimensional neutrino-radiation hydrodynamic code. The explosion is driven by the neutrino heating aided by multi-dimensional hydrodynamic effects such as the convection. Following the explosion phase, we continue the simulation focusing on the thermal evolution of the protoneutron star up to $\sim$70 s when the crust of the neutron star is formed using one-dimensional simulation. We find that the crust forms at high-density region ($\rho\sim10^{14}$ g cm$^{-3}$) and it would proceed from inside to outside. This is the first self-consistent simulation that successfully follows from the collapse phase to the protoneutron star cooling phase based on the multi-dimensional hydrodynamic simulation.
1311.7249v2
2013-12-01
Chemical Bonding in Aqueous Ferrocyanide: Experimental and Theoretical X-ray Spectroscopic Study
Resonant inelastic X-ray scattering (RIXS) and X-ray absorption (XA) experiments at the iron L- and nitrogen K-edge are combined with high-level first principles restricted active space self-consistent field (RASSCF) calculations for a systematic investigation of the nature of the chemical bond in potassium ferrocyanide in aqueous solution. The atom- and site-specific RIXS excitations allow for direct observation of ligand-to-metal (Fe L-edge) and metal-to-ligand (N K-edge) charge transfer bands and thereby evidence for strong {\sigma}-donation and {\pi}-back-donation. The effects are identified by comparing experimental and simulated spectra related to both the unoccupied and occupied molecular orbitals in solution.
1312.0236v1
2013-12-04
Ray-tracing in pseudo-complex General Relativity
Motivated by possible observations of the black hole candidate in the center of our galaxy and the galaxy M87, ray-tracing methods are applied to both standard General Relativity (GR) and a recently proposed extension, the pseudo-complex General Relativity (pc-GR). The correction terms due to the investigated pc-GR model lead to slower orbital motions close to massive objects. Also the concept of an innermost stable circular orbit (ISCO) is modified for the pc-GR model, allowing particles to get closer to the central object for most values of the spin parameter $a$ than in GR. Thus, the accretion disk, surrounding a massive object, is brighter in pc-GR than in GR. Iron K$\alpha$ emission line profiles are also calculated as those are good observables for regions of strong gravity. Differences between the two theories are pointed out.
1312.1170v2
2013-12-09
Point contact spectroscopy in Fe-based superconductors: recent advancements and future challenges
Iron-based superconductors (FeSC) present an unprecedented variety of features both in the superconducting and in the normal state. Different families differ in the value of the critical temperature, in the shape of the Fermi surface, in the existence or absence of quasi-nesting conditions, in the range of doping in which the antiferromagnetic (AFM) and the superconducting phase coexist and in the structure of the order parameter in the reciprocal space, and so on. In this paper the most important results of point-contact spectroscopy (PCS) in Fe-based superconductors are reviewed, and the most recent advances are described with the aim to discuss the future perspectives and challenges of this spectroscopic technique in the characterization of the superconducting properties of these complex compounds. One of the main challenges, faced so far only by a few researchers in the PCS field, is to fully explore the phase diagram of these materials, as a function of doping or pressure, to understand the interplay between superconductivity and magnetism, the effect of intrinsic or extrinsic inhomogeneities, the role of spin fluctuations (SFs) in the pairing, the symmetry and the structure of the order parameter(s).
1312.2527v1
2013-12-10
On the origin of variable structures in the winds of hot luminous stars
Examination of the temporal variability properties of several strong optical recombination lines in a large sample of Galactic Wolf-Rayet (WR) stars reveals possible trends, especially in the more homogeneous WC than the diverse WN subtypes, of increasing wind variability with cooler subtypes. This could imply that a serious contender for the driver of the variations is stochastic, magnetic subsurface convection associated with the 170 kK partial-ionization zone of iron, which should occupy a deeper and larger zone of greater mass in cooler WR subtypes. This empirical evidence suggests that the heretofore proposed ubiquitous driver of wind variability, radiative instabilities, may not be the only mechanism playing a role in the stochastic multiple small-scaled structures seen in the winds of hot luminous stars. In addition to small-scale stochastic behaviour, subsurface convection guided by a global magnetic field with localized emerging loops may also be at the origin of the large-scale corotating interaction regions as seen frequently in O stars and occasionally in the winds of their descendant WR stars.
1312.2864v1
2013-12-10
Spectrum splitting of bimagnon excitations in a spatially frustrated Heisenberg antiferromagnet revealed by resonant inelastic x-ray scattering
We perform a comprehensive analysis of the bimagnon resonant inelastic x-ray scattering (RIXS) intensity spectra of the spatially frustrated Jx-Jy-J2 Heisenberg model on a square lattice in both the antiferromagnetic and the collinear antiferromagnetic phase. We study the model for strong frustration and significant spatial anisotropy to highlight the key signatures of RIXS spectrum splitting which may be experimentally discernible. Based on an interacting spin wave theory study within the ladder approximation Bethe-Salpeter scheme, we find the appearance of a robust two-peak structure over a wide range of the transferred momenta in both magnetically ordered phases. The unfrustrated model has a single-peak structure with a two-peak splitting originating due to spatial anisotropy and frustrated interactions. Our predicted two-peak structure from both magnetically ordered regime can be realized in iron pnictides.
1312.2876v2
2013-12-12
Impact of electronic correlations on the equation of state and transport in $ε$-Fe
We have obtained the equilibrium volumes, bulk moduli, equations of state of the ferromagnetic cubic $\alpha$ and paramagnetic hexagonal $\epsilon$ phases of iron in close agreement with experiment using an ab initio dynamical mean-field theory approach. The local dynamical correlations are shown to be crucial for a successful description of the ground-state properties of paramagnetic $\epsilon$-Fe. Moreover, they enhance the effective mass of the quasiparticles and reduce their lifetimes across the $\alpha \to \epsilon$ transition leading to a step-wise increase of the resistivity, as observed in experiment. The calculated magnitude of the jump is significantly underestimated, which points to non-local correlations. The implications of our results for the superconductivity and non-Fermi-liquid behavior of $\epsilon$-Fe are discussed.
1312.3654v1
2013-12-13
Phosphorus in the Young Supernova Remnant Cassiopeia A
Phosphorus ($^{31}$P), which is essential for life, is thought to be synthesized in massive stars and dispersed into interstellar space when these stars explode as supernovae (SNe). Here we report on near-infrared spectroscopic observations of the young SN remnant Cassiopeia A, which show that the abundance ratio of phosphorus to the major nucleosynthetic product iron ($^{56}$Fe) in SN material is up to 100 times the average ratio of the Milky Way, confirming that phosphorus is produced in SNe. The observed range is compatible with predictions from SN nucleosynthetic models but not with the scenario in which the chemical elements in the inner SN layers are completely mixed by hydrodynamic instabilities during the explosion.
1312.3807v1
2013-12-16
Optical conductivity of nodal metals
Fermi liquid theory is remarkably successful in describing the transport and optical properties of metals; at frequencies higher than the scattering rate, the optical conductivity adopts the well-known power law behavior $\sigma_1(\omega) \propto \omega^{-2}$. We have observed an unusual non-Fermi liquid response $\sigma_1(\omega) \propto \omega^{-1\pm 0.2}$ in the ground states of several cuprate and iron-based materials which undergo electronic or magnetic phase transitions resulting in dramatically reduced or nodal Fermi surfaces. The identification of an inverse (or fractional) power-law behavior in the residual optical conductivity now permits the removal of this contribution, revealing the direct transitions across the gap and allowing the nature of the electron-boson coupling to be probed. The non-Fermi liquid behavior in these systems may be the result of a common Fermi surface topology of Dirac cone-like features in the electronic dispersion.
1312.4466v1
2013-12-20
Ultrafast modulation of the chemical potential in BaFe$_2$As$_2$ by coherent phonons
Time- and angle-resolved extreme ultraviolet photoemission spectroscopy is used to study the electronic structure dynamics in BaFe$_2$As$_2$ around the high-symmetry points $\Gamma$ and $M$. A global oscillation of the Fermi level at the frequency of the $A_{1g}$(As) phonon mode is observed. It is argued that this behavior reflects a modulation of the effective chemical potential in the photoexcited surface region that arises from the high sensitivity of the band structure near the Fermi level to the $A_{1g}$ phonon mode combined with a low electron diffusivity perpendicular to the layers. The results establish a novel way to tune the electronic properties of iron pnictides: coherent control of the effective chemical potential. The results further suggest that the equilibration time for the effective chemical potential needs to be considered in the ultrafast electronic structure dynamics of materials with weak interlayer coupling.
1312.6025v1
2013-12-23
Heat capacity jump at T_c and pressure derivatives of superconducting transition temperature in the Ba(1-x)NaxFe2As2 (0.1 <= x <= 0.9) series
We present the evolution of the initial (up to ~ 10 kbar) hydrostatic, pressure dependencies of T_c and of the ambient pressure jump in the heat capacity associated with the superconducting transition as a function of Na - doping in the Ba(1-x)NaxFe2As2 family of iron-based superconductors. For Na concentrations 0.15 <= x <= 0.9, the jump in specific heat at T_c, Delta C_p, follows the Delta C_p ~ T^3 scaling found for most BaFe2As2 - based superconductors. Pressure dependencies are non-monotonic for x = 0.2 and x = 0.24. For other Na concentrations T_c decreases under pressure in almost linear fashion. The anomalous behavior of the x = 0.2 and x = 0.24 samples under pressure are possibly due to the crossing of the phase boundaries of the narrow antiferromagnetic tetragonal phase, unique for the Ba(1-x)NaxFe2As2 series, with the application of pressure.
1312.6705v1
2014-01-07
The polluted atmospheres of cool white dwarfs and the magnetic field connection
We present an analysis of X-Shooter spectra of the polluted hydrogen-rich white dwarfs (DAZ) NLTT 888 and NLTT 53908. The spectra of NLTT 53908 show strong, Zeeman-split calcium lines (CaII H&K and Ca I $\lambda 4226$) and the star appears to be a close relative of the polluted magnetic white dwarf (DAZH) NLTT 10480, while the spectra of NLTT 888 show narrow lines of calcium and iron. A comparison of the DAZ NLTT 888 and the DAZH NLTT 53908 with other class members illustrates the diversity of environment and formation circumstances surrounding these objects. In particular, we find that the incidence of magnetism in old, polluted white dwarfs significantly exceeds that found in the general white dwarf population which suggests an hypothetical link between a crowded planetary system and magnetic field generation.
1401.1249v1
2014-01-10
The Iron K Line Profile of IRAS 18325-5926
IRAS 18325-5926 is an X-ray bright, Compton-thin, type-2 Seyfert galaxy and it was the first Seyfert 2 in which the presence of a broad Fe K-alpha emission line was claimed. However, although the structure of the Fe line appears broad, there is tentative evidence that it may comprise multiple lines. Nevertheless, previous analyses have only consisted of fitting standalone broad components to the Fe K band. Here, we have analyzed all available X-ray CCD data from Suzaku, XMM-Newton and ASCA to fully investigate the nature of the emission complex by testing broad-band physical models and alternative hypotheses. We find that both a model consisting of broad, blurred reflection from an ionized accretion disc and a model consisting of cold, neutral reflection plus narrow emission lines from highly-ionized photoionized gas (log \xi = 3.5) offer statistically comparable fits to the data although the true reality of the Fe line cannot currently be determined with existing data. However, it is hoped that better quality data and improved photon statistics in the Fe K band will allow a more robust distinction between models to be made.
1401.2420v1
2014-01-14
Ipopv2: Photoionization of Ni XIV -- a test case
Several years ago, M. Asplund and coauthors (2004) proposed a revision of the Solar composition. The use of this new prescription for Solar abundances in standard stellar models generated a strong disagreement between the predictions and the observations of Solar observables. Many claimed that the Standard Solar Model (SSM) was faulty, and more specifically the opacities used in such models. As a result, activities around the stellar opacities were boosted. New experiments (J. Bailey at Sandia on Z-Pinch, The OPAC consortium at LULI200) to measure directly absorbtion coefficients have been realized or are underway. Several theoretical groups (CEA-OPAS, Los Alamos Nat. Lab., CEA-SCORCG, The Opacity Project - The Iron Project (IPOPv2)) have started new sets of calculations using different approaches and codes. While the new results seem to confirm the good quality of the opacities used in SSM, it remains important to improve and complement the data currently available. We present recent results in the case of the photoionization cross sections for Ni XIV (Ni13+ ) from IPOPv2 and possible implications on stellar modelling.
1401.3122v1
2014-01-16
Terzan 5: a pristine fragment of the Galactic Bulge?
Terzan 5 is a stellar system located in the inner Bulge of the Galaxy and has been historically catalogued as a globular cluster. However, recent photometric (Ferraro et al. 2009) and spectroscopic (Origlia et al. 2011; Origlia et al. 2013) investigations have shown that it hosts at least three stellar populations with different iron abundances (with a total spread of Delta[Fe/H]>1 dex) thus demonstrating that Terzan 5 is not a genuine globular cluster. In addition, the striking similarity between the chemical patterns of this system and those of its surrounding environment, the Galactic Bulge, from the point of view of both the metallicity distribution and the alpha-element enrichment, suggests that Terzan 5 could be a pristine fragment of the Bulge itself.
1401.3962v1
2014-01-20
Total and Partial Fragmentation Cross-Section of 500 MeV/nucleon Carbon Ions on Different Target Materials
By using an experimental setup based on thin and thick double-sided microstrip silicon detectors, it has been possible to identify the fragmentation products due to the interaction of very high energy primary ions on different targets. Here we report total and partial cross-sections measured at GSI (Gesellschaft fur Schwerionenforschung), Darmstadt, for 500 MeV/n energy $^{12}C$ beam incident on water (in flasks), polyethylene, lucite, silicon carbide, graphite, aluminium, copper, iron, tin, tantalum and lead targets. The results are compared to the predictions of GEANT4 (v4.9.4) and FLUKA (v11.2) Monte Carlo simulation programs.
1401.4897v1
2014-01-21
Tunable VUV laser based spectrometer for Angle Resolved Photoemission Spectroscopy (ARPES)
We have developed an angle-resolved photoemission spectrometer with tunable VUV laser as a photon source. The photon source is based on the fourth harmonic generation of a near IR beam from a Ti:sapphire laser pumped by a CW green laser and tunable between 5.3eV and 7eV. The most important part of the set-up is a compact, vacuum enclosed fourth harmonic generator based on KBBF crystals, grown hydrothermally in the US. This source can deliver a photon flux of over 10^14 photons/s. We demonstrate that this energy range is sufficient to measure the kz dispersion in an iron arsenic high temperature superconductor, which was previously only possible at synchrotron facilities.
1401.5404v1
2014-01-21
Dramatic Changes in the Electronic Structure Upon Transition to the Collapsed Tetragonal Phase in CaFe2As2
We use angle-resolved photoemission spectroscopy (ARPES) and density functional theory (DFT) calculations to study the electronic structure of CaFe$_2$As$_2$ in previously unexplored collapsed tetragonal (CT) phase. This unusual phase of the iron arsenic high temperature superconductors was hard to measure as it exists only under pressure. By inducing internal strain, via the post growth, thermal treatment of the single crystals, we were able to stabilize the CT phase at ambient-pressure. We find significant differences in the Fermi surface topology and band dispersion data from the more common orthorhombic-antiferromagnetic or tetragonal-paramagnetic phases, consistent with electronic structure calculations. The top of the hole bands sinks below the Fermi level, which destroys the nesting present in parent phases. The absence of nesting in this phase along with apparent loss of Fe magnetic moment, are now clearly experimentally correlated with the lack of superconductivity in this phase.
1401.5416v1
2014-01-22
The effect of exceptionally high fluorine doping on the anisotropy of single crystalline SmFeAsO1-xFx
We succeeded in growing single crystalline SmFeAsO1-xFx with exceptionally high fluorine concentration by using a CsCl flux method. Comparing to conventional flux methods, this method can introduce about double the amount of fluorine into the oxygen site. The obtained single crystal shows the highest superconducting transition temperature (Tc = 57.5 K) in single crystalline iron pnictides. In addition, the residual resistivity ratio (RRR) is almost three times as large as that of previously reported single crystals. This suggests that our single crystals are suitable for investigation of the intrinsic superconducting properties since they have few defects and impurities. Using both the Werthamer-Helfand-Hohenberg model and the effective mass model, we demonstrated that a higher fluorine concentration suppresses the anisotropic superconductivity of SmFeAsO1-xFx.
1401.5611v2
2014-01-28
Phase Transformation Dynamics in Porous Battery Electrodes
Porous electrodes composed of multiphase active materials are widely used in Li-ion batteries, but their dynamics are poorly understood. Two-phase models are largely empirical, and no models exist for three or more phases. Using a modified porous electrode theory based on non-equilibrium thermodynamics, we show that experimental phase behavior can be accurately predicted from free energy models, without artificially placing phase boundaries or fitting the open circuit voltage. First, we simulate lithium intercalation in porous iron phosphate, a popular two-phase cathode, and show that the zero-current voltage gap, sloping voltage plateau and under-estimated exchange currents all result from size-dependent nucleation and mosaic instability. Next, we simulate porous graphite, the standard anode with three stable phases, and reproduce experimentally observed fronts of color-changing phase transformations. These results provide a framework for physics-based design and control for electrochemical systems with complex thermodynamics.
1401.7072v2
2014-01-29
The poisoning effect of Mn in LaFe(1-x)Mn(x)AsO(0.89)F(0.11): unveiling a quantum critical point in the phase diagram of iron-based superconductors
A superconducting-to-magnetic transition is reported for LaFe$_{1-x}$Mn$_x$AsO$_{0.89}$F$_{0.11}$ where a per thousand amount of Mn impurities is dispersed. By employing local spectroscopic techniques like muon spin rotation (muSR) and nuclear quadrupole resonance (NQR) on compounds with Mn contents ranging from x=0.025% to x=0.75%, we find that the electronic properties are extremely sensitive to the Mn impurities. In fact, a small amount of Mn as low as 0.2% suppresses superconductivity completely. Static magnetism, involving the FeAs planes, is observed to arise for x > 0.1% and becomes further enhanced upon increasing Mn substitution. Also a progressive increase of low energy spin fluctuations, leading to an enhancement of the NQR spin-lattice relaxation rate 1/T1, is observed upon Mn substitution. The analysis of 1/T1 for the sample closest to the the crossover between superconductivity and magnetism (x = 0.2%) points towards the presence of an antiferromagnetic quantum critical point around that doping level.
1401.7576v1
2014-01-30
Electronic structure of BaNi$_2$P$_2$ observed by angle-resolved photoemission spectroscopy
We have performed an angle-resolved photoemission spectroscopy (ARPES) study of BaNi$_2$P$_2$ which shows a superconducting transition at $T_c$ $\sim$ 2.5 K. We observed hole and electron Fermi surfaces (FSs) around the Brillouin zone center and corner, respectively, and the shapes of the hole FSs dramatically changed with photon energy, indicating strong three-dimensionality. The observed FSs are consistent with band-structure calculation and de Haas-van Alphen measurements. The mass enhancement factors estimated in the normal state were $m^*$/$m_b$ $\leq$ 2, indicating weak electron correlation compared to typical iron-pnictide superconductors. An electron-like Fermi surface around the Z point was observed in contrast with BaNi$_2$As$_2$ and may be related to the higher $T_c$ of BaNi$_2$P$_2$.
1401.7897v2
2014-01-31
A global cloud map of the nearest known brown dwarf
Brown dwarfs -- substellar bodies more massive than planets but not massive enough to initiate the sustained hydrogen fusion that powers self-luminous stars -- are born hot and slowly cool as they age. As they cool below about 2,300 K, liquid or crystalline particles composed of calcium aluminates, silicates and iron condense into atmospheric 'dust', which disappears at still cooler temperatures (around 1,300 K). Models to explain this dust dispersal include both an abrupt sinking of the entire cloud deck into the deep, unob- servable atmosphere and breakup of the cloud into scattered patches (as seen on Jupiter and Saturn). Thus far, observations of brown dwarfs have been limited to globally integrated measurements, which can reveal surface inhomogeneities but cannot unambiguously resolve surface features. Here we report a two-dimensional map of a brown dwarf's surface that allows identification of large-scale bright and dark features, indicative of patchy clouds.
1401.8145v1
2014-02-01
Phase stability and Nucleation effect upon Iron addition to SmCo5 bulk magnets
Change in structure and magnetic properties of SmCo5-xFex permanent magnets for different values of x ranging from 0 to 2 have been studied. Structural investigation from X-ray diffraction (XRD) patterns confirms the hexagonal CaCu5-type structure of the SmCo5-xFex ribbons for 0<x<2. The decrease in angular position of the diffraction peaks points to the lattice expansion due to the substitution of Co atoms by larger Fe atoms. Mixture of phases occurs for x>2 and has been confirmed by both XRD studies and magnetic measurements. Nucleation effect induced by the additive Fe enhances the coercivity (Hc)up to 27 kOe which is much larger than 4.5 kOe obtained for pure SmCo5.
1402.0138v1
2014-02-03
Hemispherical Parker waves driven by thermal shear in planetary dynamos
Planetary and stellar magnetic fields are thought to be sustained by helical motions ($\alpha$-effect) and, if present, differential rotation ($\Omega$-effect). In the Sun, the strong differential rotation in the tachocline is responsible for an efficient $\Omega$-effect creating a strong axisymmetric azimuthal magnetic field. This is a prerequisite for Parker dynamo waves that may be responsible for the solar cycle. In the liquid iron cores of terrestrial planets, the Coriolis force organizes convection into columns with a strong helical flow component. These likely dominate magnetic field generation while the $\Omega$-effect is of secondary importance. Here we use numerical simulations to show that the planetary dynamo scenario may change when the heat flux through the outer boundary is higher in one hemisphere than in the other. A hemispherical dynamo is promoted that is dominated by fierce thermal wind responsible for a strong $\Omega$-effect. As a consequence Parker dynamo waves are excited equivalent to those predicted for the Sun. They obey the same dispersion relation and propagation characteristics. We suggest that Parker waves may therefore also play a role in planetary dynamos for all scenarios where zonal flows become an important part of convective motions.
1402.0343v1
2014-02-06
Temperature-induced Change in the Fermi Surface Topology in the Spin Density Wave Phase of Sr(Fe$_{1-x}$Co$_x$)$_2$As$_2$
We report electronic Raman scattering measurements of Sr(Fe$_{1-x}$Co$_x$)$_2$As$_2$ single crystals in their magnetic - Spin Density Wave (SDW) phase. The spectra display multiple, polarization-resolved SDW gaps as expected in a band-folding itinerant picture for a multiband system. The temperature dependence of the SDW gaps reveals an unusual evolution of the reconstructed electronic structure with at least one gap being activated only well below the magnetic SDW transition $T_N$. A comparison with temperature dependent Hall measurements allows us to assign this activated behavior to a change in the Fermi surface topology deep in the SDW phase, which we attribute to the disappearance of a hole-like Fermi pocket. Our results highlight the strong sensitivity of the low energy electronic structure to temperature in iron-arsenide superconductors.
1402.1422v2
2014-02-07
Signatures of superconducting and pseudogap phases in ultrafast transient reflectivity of Ca(Fe0.927Co0.073)2As2
We present femtosecond time-resolved pump-probe spectroscopic studies of a pseudogap (PG) along with the superconducting (SC) gap in an overdoped iron pnictide Ca(Fe0.927Co0.073)2As2. It is seen that the temperature evolution of the photoexcited quasiparticle (QP) relaxation dynamics, coherently excited A1g-symmetric optical phonon and two acoustic phonon dynamics behave anomalously in the vicinity of the superconducting transition temperature Tc. A continuous change in the sign of the experimentally measured transient differential reflectivity Delta_R/R signal at the zero time-delay between the pump and probe pulses at a temperature of ~200 K is inferred as an evidence of the emergence of the PG phase around that temperature. This behavior is independent of the pump photon energy and occurs for crystals without the spin density wave phase transition.
1402.1627v1
2014-02-07
Suzaku Discovery of Fe K-Shell Line from the O-Rich SNR G292.0+1.8
We report the Suzaku/XIS results of the Galactic oxygen-rich supernova remnant (SNR), G292.0+1.8, a remnant of a core-collapse supernova. The X-ray spectrum of G292.0+1.8 consists of two type plasmas, one is in collisional ionization equilibrium (CIE) and the other is in non-equilibrium ionization (NEI). The CIE plasma has nearly solar abundances, and hence would be originated from the circumstellar and interstellar mediums. The NEI plasma has super-solar abundances, and the abundance pattern indicates that the plasma originates from the supernova ejecta with a main sequence of 30-35 Msolar. Iron K-shell line at energy of 6.6 keV is detected for the first time in the NEI plasma.
1402.1633v1
2014-02-12
Electron Impact Ionization of Stored Highly Charged Ions
Accurate cross section data for electron impact ionization (EII) are needed in order to interpret the spectra of collisionally ionized plasmas both in astrophysics and in the laboratory. Models and spectroscopic diagnostics of such plasmas rely on accurate ionization balance calculations, which depend, in turn, on the underlying rates for EII and electron-ion recombination. EII measurements have been carried out using the TSR storage ring located at the Max-Planck-Institut fuer Kernphysik in Heidelberg, Germany. Storage ring measurements are largely free of metastable contamination, resulting in unambiguous EII data, unlike what is encountered with other experimental geometries. As it is impractical to perform experiments for every ion, theory must provide the bulk of the necessary EII data. In order to guide theory, TSR experiments have focused on providing at least one measurement for every isoelectronic sequence. EII data have been measured for ions from 13 isoelectronic sequences: Li-like silicon and chlorine, Be-like sulfur, B-like magnesium, and F-like through K-like iron. These experimental results provide an important benchmark for EII theory.
1402.2964v1
2014-02-21
Enhancement of Superconducting Transition Temperature Due to Antiferromagnetic Spin Fluctuations in Iron-pnictides LaFe(As_{1-x}P_x)(O_{1-y}F_y) : 31P-NMR Studies
Systematic P-NMR studies on LaFe(As_{1-x}P_x)(O_{1-y}F_y) with y=0.05 and 0.1 have revealed that the antiferromagnetic spin fluctuations (AFMSFs) at low energies are markedly enhanced around x=0.6 and 0.4, respectively, and as a result, Tc exhibits respective peaks at 24 K and 27 K against the P-substitution for As. This result demonstrates that the AFMSFs are responsible for the increase in Tc for LaFe(As_{1-x}P_x)(O_{1-y}F_y) as a primary mediator of the Cooper pairing. From a systematic comparison of AFMSFs with a series of (La_{1-z}Y_z)FeAsO_{\delta} compounds in which Tc reaches 50 K for z=0.95, we remark that a moderate development of AFMSFs causes the Tc to increase up to 50 K under the condition that the local lattice parameters of FeAs tetrahedron approaches those of the regular tetrahedron. We propose that the T_c of Fe-pnictides exceeding 50 K is maximized under an intimate collaboration of the AFMSFs and other factors originating from the optimization of the local structure.
1402.5220v1
2014-03-02
Transport in multiband systems with hot spots on the Fermi surface: Forward-scattering corrections
Multiband models with hot spots are of current interest partly because of their relevance for the iron-based superconductors. In these materials, the momentum-dependent scattering off spin fluctuations and the ellipticity of the electron Fermi pockets are responsible for anisotropy of the lifetimes of excitations around the Fermi surface. The deep minima of the lifetimes---the so-called hot spots---have been assumed to contribute little to the transport as is indeed predicted by a simple relaxation-time approach. Calculating forward-scattering corrections to this approximation, we find that the effective transport times are much more isotropic than the lifetimes and that, therefore, the hot spots contribute to the transport even in the case of strong spin-fluctuation scattering. We discuss this effect on the basis of an analytical solution of the Boltzmann equation and calculate numerically the temperature and doping dependence of the resistivity and the Hall, Seebeck, and Nernst coefficients.
1403.0144v2
2014-03-02
Heat transport in RbFe2As2 single crystal: evidence for nodal superconducting gap
The in-plane thermal conductivity of iron-based superconductor RbFe$_2$As$_2$ single crystal ($T_c \approx$ 2.1 K) was measured down to 100 mK. In zero field, the observation of a significant residual linear term $\kappa_0/T$ = 0.65 mW K$^{-2}$ cm$^{-1}$ provides clear evidence for nodal superdonducting gap. The field dependence of $\kappa_0/T$ is similar to that of its sister compound CsFe$_2$As$_2$ with comparable residual resistivity $\rho_0$, and lies between the dirty and clean KFe$_2$As$_2$. These results suggest that the (K,Rb,Cs)Fe$_2$As$_2$ serial superconductors have a common nodal gap structure.
1403.0191v3
2014-03-02
Nodeless superconducting gaps in Ca$_{10}$(Pt$_{4-δ}$As$_8$)((Fe$_{1-x}$Pt$_{x}$)$_2$As$_2$)$_5$ probed by quasiparticle heat transport
The in-plane thermal conductivity of iron-based superconductor Ca$_{10}$(Pt$_{4-\delta}$As$_8$)((Fe$_{1-x}$Pt$_{x}$)$_2$As$_2$)$_5$ single crystal (``10-4-8", $T_c$ = 22 K) was measured down to 80 mK. In zero field, the residual linear term $\kappa_0/T$ is negligible, suggesting nodeless superconducting gaps in this multiband compound. In magnetic fields, $\kappa_0/T$ increases rapidly, which mimics those of multiband superconductor NbSe$_2$ and LuNi$_2$B$_2$C with highly anisotropic gap. Such a field dependence of $\kappa_0/T$ is an evidence for multiple superconducting gaps with quite different magnitudes or highly anisotropic gap. Comparing with the London penetration depth results of Ca$_{10}$(Pt$_3$As$_8$)((Fe$_{1-x}$Pt$_{x}$)$_2$As$_2$)$_5$ (``10-3-8") compound, the 10-4-8 and 10-3-8 compounds may have similar superconducting gap structure.
1403.0194v1
2014-03-04
Tunnel diode oscillator measurements of the upper critical magnetic field of FeTe0:5Se0:5
Temperature dependence of the upper critical magnetic field (Hc2) of single crystalline FeTe0.5Se0.5 (Tc = 14.5 K) have been determined by tunnel diode oscillator-based measurements in magnetic fields of up to 55 T and temperatures down to 1.6 K. The Werthamer-Helfand-Hohenberg model accounts for the data for magnetic field applied both parallel (H || ab) and perpendicular (H || c) to the iron conducting plane, in line with a single band superconductivity. Whereas Pauli pair breaking is negligible for H || c, Pauli contribution is evidenced for H || ab with Maki parameter alpha= 1.4, corresponding to Pauli field HP = 79 T. As a result, the Hc2 anisotropy (= Habc2 /Hcc2) which is already rather small at Tc (gamma = 1.6) further decreases as the temperature decreases and becomes smaller than 1 at liquid helium temperatures.
1403.0844v1
2014-03-05
Design and demonstration of a quasi-monoenergetic neutron source
The design of a neutron source capable of producing 24 and 70 keV neutron beams with narrow energy spread is presented. The source exploits near-threshold kinematics of the $^{7}$Li(p,n)$^{7}$Be reaction while taking advantage of the interference `notches' found in the scattering cross-sections of iron. The design was implemented and characterized at the Center for Accelerator Mass Spectrometry at Lawrence Livermore National Laboratory. Alternative filters such as vanadium and manganese are also explored and the possibility of studying the response of different materials to low-energy nuclear recoils using the resultant neutron beams is discussed.
1403.1285v2
2014-03-08
High critical-current density with less anisotropy in BaFe2(As,P)2 epitaxial thin films: Effect of intentionally grown c-axis vortex-pinning centers
We report herein a high and isotropic critical-current density Jc for BaFe2(As,P)2 epitaxial films. The isotropy of Jc with respect to the magnetic-field direction was improved significantly by decreasing the film growth rate to 2.2 {\AA}/s. The low growth rate served to preferentially align dislocations along the c-axis, which work well as c-axis vortex-pinning centers. Because of the intentional introduction of effective pinning, the absolute Jc at 9 T was larger than that obtained for other iron-based superconductors and conventional alloy superconducting wires.
1403.1947v2
2014-03-08
Challenges in nucleosynthesis of trans-iron elements
Nucleosynthesis beyond Fe poses additional challenges not encountered when studying astrophysical processes involving light nuclei. Astrophysical sites and conditions are not well known for some of the processes involved. On the nuclear physics side, different approaches are required, both in theory and experiment. The main differences and most important considerations are presented for a selection of nucleosynthesis processes and reactions, specifically the $s$-, $r$-, $\gamma$-, and $\nu p$-processes. Among the discussed issues are uncertainties in sites and production conditions, the difference between laboratory and stellar rates, reaction mechanisms, important transitions, thermal population of excited states, and uncertainty estimates for stellar rates. The utility and limitations of indirect experimental approaches are also addressed. The presentation should not be viewed as confining the discussed problems to the specific processes. The intention is to generally introduce the concepts and possible pitfalls along with some examples. Similar problems may apply to further astrophysical processes involving nuclei from the Fe region upward and/or at high plasma temperatures. The framework and strategies presented here are intended to aid the conception of future experimental and theoretical approaches.
1403.2015v1
2014-03-11
Chemical abundance analysis of symbiotic giants. I. RW Hya and SY Mus
The study of symbiotic systems is of considerable importance in our understanding of binary system stellar evolution in systems where mass loss or transfer takes place. Elemental abundances are of special significance since they can be used to track mass exchange. However, there are few symbiotic giants for which the abundances are fairly well determined. Here we present for the first time a detailed analysis of the chemical composition for the giants in the RW Hya and SY Mus systems. The analysis is based on high resolution (R 50000), high S/N, near-IR spectra. Spectrum synthesis employing standard LTE analysis and atmosphere models was used to obtain photospheric abundances of CNO and elements around the iron peak (Sc, Ti, Fe, and Ni). Our analysis reveals a significantly sub-solar metallicity, [Fe/H]-0.75}, for the RW Hya giant confirming its membership in the Galactic halo population and a near-solar metallicity for the SY Mus giant. The very low 12C/13C isotopic ratios, 6-10, derived for both objects indicate that the giants have experienced the first dredge-up
1403.2659v1
2014-03-22
Neutron Reactions in Astrophysics
The quest for the origin of matter in the Universe had been the subject of philosophical and theological debates over the history of mankind, but quantitative answers could be found only by the scientific achievements of the last century. A first important step on this way was the development of spectral analysis by Kirchhoff and Bunsen in the middle of the 19$^{\rm th}$ century, which provided first insight in the chemical composition of the sun and the stars. The energy source of the stars and the related processes of nucleosynthesis, however, could be revealed only with the discoveries of nuclear physics. A final breakthrough came eventually with the compilation of elemental and isotopic abundances in the solar system, which are reflecting the various nucleosynthetic processes in detail. This review is focusing on the mass region above iron, where the formation of the elements is dominated by neutron capture, mainly in the slow ($s$) and rapid ($r$) processes. Following a brief historic account and a sketch of the relevant astrophysical models, emphasis is put on the nuclear physics input, where status and perspectives of experimental approaches are presented in some detail, complemented by the indispensable role of theory.
1403.5670v1
2014-03-24
Dust formation in macronovae
We examine dust formation in macronovae (as known as kilonovae), which are the bright ejecta of neutron star binary mergers and one of the leading sites of r-process nucleosynthesis. We find that dust grains of r-process elements are difficult to form because of the low number density of the r-process atoms, while carbon or elements lighter than irons can condense into dust if they are abundant, in light of the first macronova candidate associated with GRB 130603B. Dust grains absorb emission from ejecta with opacity even greater than that of the r-process elements, and re-emit photons at infrared wavelengths. Such dust emission can potentially account for the macronova without r-process nucleosynthesis as an alternative model. This dust scenario predicts a more featureless spectrum than the r-process model and day-scale optical-to-ultraviolet emission.
1403.5872v2
2014-03-26
Photoconductivity and photo-detection response of multiferroic bismuth iron oxide
We report visible light detection with in-plane BiFeO3 (BFO) thin films grown on pre-patterned inter-digital electrodes. In-plane configured BFO film displayed photocurrents with a 40:1 photo-to-dark-current ratio and improved photo-sensing ability for >15000 s (4 hrs) under small bias voltage (42V). Nearly sixty percent of the photo-induced charge carriers decay in 1.0 s and follow a double-exponential decay model. At 373 K the effect of light does not significantly increase the dark current, probably due to reduced mobility. Sub-bandgap weak monochromatic light (1 mw/cm2) shows one fold increase in photo-charge carriers.
1403.6748v1
2014-03-26
Simulating a two-dimensional frustrated spin system with fermionic resonating-valence-bond states
The frustrated Heisenberg $J_{1}-J_{2}$ model on a square lattice is numerically investigated by variational Monte Carlo simulations. We propose a antiferromagnetic fermion resonating-valence-bond (AF-fRVB) state that has ability to examine the entire phase diagram in the $J_{1}-J_{2}$ model. Two phase transition points, the second order around $J_{2}/J_{1}=0.45$ and the first order around $J_{2}/J_{1}=0.6$, can be extracted more clearly than the conventional bosonic RVB state. At the maximally frustrated point ($J_{2}/J_{1}=0.5$), the AF-fRVB state shows the variational ground-state energy in the thermodynamic limit very close to the one estimated by the projected entangled pair state at the largest bond dimension available. On the other hand, in the frustrated regime $0.4\lesssim J_{2}/J_{1}\leq0.5$, AF-fRVB states with $s_{+-}$ (using the terminology in the field of iron-based superconductors) and $d_{xy}$ pairing symmetries are degenerate in the thermodynamic limit, implying the existence of gapless Dirac excitations in the spinon spectrum.
1403.6879v1
2014-03-30
Scattering of electron vortex beams on a magnetic crystal: towards atomic resolution magnetic measurements
Use of electron vortex beams (EVB), that is convergent electron beams carrying an orbital angular momentum (OAM), is a novel development in the field of transmission electron microscopy. They should allow measurement of element-specific magnetic properties of thin crystals using electron magnetic circular dichroism (EMCD)---a phenomenon similar to the x-ray magnetic circular dichroism. Recently it has been shown computationally that EVBs can detect magnetic signal in a scanning mode only at atomic resolution. In this follow-up work we explore in detail the elastic and inelastic scattering properties of EVBs on crystals, as a function of beam diameter, initial OAM, acceleration voltage and beam displacement from an atomic column. We suggest that for a 10 nm layer of bcc iron oriented along (001) zone axis an optimal configuration for a detection of EMCD is an EVB with OAM of $1\hbar$ and a diameter of 1.6 \AA, acceleration voltage 200 keV and an annular detector with inner and outer diameters of $G$ and $5G$, respectively, where $\mathbf{G}=(100)$.
1403.7730v1
2014-03-31
Strain effects on electronic structure and superconductivity in the iron telluride
The influence of tensile strain in the ab-plane on crystal and electronic structure of FeTe has been studied ab initio. In superconducting FeSe the Fermi surface nesting with a vector q~(0.5,0.5)(2\pi /a) is believed to be crucial for rising superconductivity mediated by spin-fluctuations. The results presented here indicate that tensile-strained FeTe also exhibits such conditions. Furthermore, the Fermi surface changes, related to the increase of the lattice parameter a of this telluride, are opposite to analogous effects reported for FeSe. Since a recently reported transition from the double-stripe to the single-stripe magnetic order in FeTe under tensile strain in the ab-plane is associated with an occurence of superconductivity in corresponding thin films, these findings allow for drawing a consistent picture of superconductivity in FeSe(1-x)Te(x) systems, in general.
1403.8005v2
2014-04-02
Spurious peaks arising from multiple scattering events involving cryostat walls in inelastic neutron scattering
Well defined peaks with energies of about 18 meV have been observed in a variety of inelastic neutron scattering experiments on single crystals as well as on powders of iron-based superconductors and their parent compounds using either the triple-axis or the time-of-flight technique. They can easily be mistaken for signatures of real excitations. We have found that they are due to multiple scattering events involving primarily walls of the sample environment. Hence, they are particularly troublesome in experiments using very small samples as have been used with recently developed high intensity neutron spectrometers. It will be discussed what needs to be done to reduce the unwanted scattering to a minimum.
1404.0522v2
2014-04-03
Charge Transfer Kinetics at the Solid-Solid Interface in Porous Electrodes
Interfacial charge transfer is widely assumed to obey Butler-Volmer kinetics. For certain liquid-solid interfaces, Marcus-Hush-Chidsey theory is more accurate and predictive, but it has not been applied to porous electrodes. Here we report a simple method to extract the charge transfer rates in carbon-coated LiFePO4 porous electrodes from chronoamperometry experiments, obtaining curved Tafel plots that contradict the Butler-Volmer equation but fit the Marcus-Hush-Chidsey prediction over a range of temperatures. The fitted reorganization energy matches the Born solvation energy for electron transfer from carbon to the iron redox site. The kinetics are thus limited by electron transfer at the solid-solid (carbon-LixFePO4) interface, rather than by ion transfer at the liquid-solid interface, as previously assumed. The proposed experimental method generalizes Chidsey's method for phase-transforming particles and porous electrodes, and the results show the need to incorporate Marcus kinetics in modeling batteries and other electrochemical systems.
1404.0859v1
2014-04-03
Fermi-Surface Reconstruction and Complex Phase Equilibria in CaFe$_{2}$As$_{2}$
Fermi-surface topology governs the relationship between magnetism and superconductivity in iron-based materials. Using low-temperature transport, angle-resolved photoemission, and x-ray diffraction we show unambiguous evidence of large Fermi surface reconstruction in CaFe$_{2}$As$_{2}$ at magnetic spin-density-wave and nonmagnetic collapsed-tetragonal ($cT$) transitions. For the $cT$ transition, the change in the Fermi surface topology has a different character with no contribution from the hole part of the Fermi surface. In addition, the results suggest that the pressure effect in CaFe$_{2}$As$_{2}$ is mainly leading to a rigid-band-like change of the valence electronic structure. We discuss these results and their implications for magnetism and superconductivity in this material.
1404.1095v1
2014-04-07
Fingerprints of Galactic Loop I on the Cosmic Microwave Background
We investigate possible imprints of galactic foreground structures such as the "radio loops" in the derived maps of the cosmic microwave background. Surprisingly there is evidence for these not only at radio frequencies through their synchrotron radiation, but also at microwave frequencies where emission by dust dominates. This suggests the mechanism is magnetic dipole radiation from dust grains enriched by metallic iron or ferrimagnetic materials. This new foreground we have identified is present at high galactic latitudes, and potentially dominates over the expected $B$-mode polarization signal due to primordial gravitational waves from inflation.
1404.1899v3
2014-04-09
Zinc abundances of planetary nebulae
Zinc is a useful surrogate element for measuring Fe/H as, unlike iron, it is not depleted in the gas phase media. Zn/H and O/Zn ratios have been derived using the [Zn IV] emission line at 3.625um for a sample of nine Galactic planetary nebulae, seven of which are based upon new observations using the VLT. Based on photoionization models, O/O++ is the most reliable ionisation correction factor for zinc that can readily be determined from optical emission lines, with an estimated accuracy of 10% or better for all targets in our sample. The majority of the sample is found to be sub-solar in [Zn/H]. [O/Zn] in half of the sample is found to be consistent with Solar within uncertainties, whereas the remaining half are enhanced in [O/Zn]. [Zn/H] and [O/Zn] as functions of Galactocentric distance have been investigated and there is little evidence to support a trend in either case.
1404.2524v1
2014-04-10
Synthesis and physical properties of Ca1-xRExFeAs2 with RE = La ~ Gd
Synthesis of a series of layered iron arsenides Ca1-xRExFeAs2 (112) was attempted by heating at 1000 C under a high-pressure of 2 GPa. The 112 phase successfully forms with RE = La, Ce, Nd, Sm, Eu and Gd, while Tb, Dy and Ho substituted and RE free samples does not contain the 112 phase. The Ce, Nd, Sm, Eu and Gd doped Ca1-xRExFeAs2 are new compounds. All of them exhibit superconducting transition except for the Ce doped sample. The behaviour of the critical temperature, with the RE ionic radii have been investigated.
1404.2738v1
2014-04-24
Superconductivity driven by the screening of long-distance Coulomb interaction
The pair-fluctuation contribution reduces the electrostatic screening length in superconductivity as compared to the normal state. When a conductor possesses a static background charge distribution, superconductivity arises even in the absence of an explicit pairing interaction, such that the Coulomb repulsion is reduced and the total energy is lowered. We demonstrate that the superconducting gap increases with increased background charge at first, after which the mixing of the Higgs and plasma modes suppresses superconductivity in the pseudogap phase. This indicates that the mechanism may be relevant to the cuprates and iron pnictides. When the background charge is identified with the incoherent component of optical conductivity in the cuprates, our results reproduce the shape, size and position of the superconducting dome with zero free parameters. A superconducting critical temperature of about 1000 K is possible in ion-doped conductors.
1404.6292v1
2014-04-25
An all-electrical torque differential magnetometer operating under ambient conditions
An all-electrical torque differential magnetometry (also known as cantilever magnetometry) setup employing piezoelectric quartz tuning forks is demonstrated. The magnetometer can be operated under ambient conditions as well as low temperatures and pressures. It extends the allowed specimen mass range up to several 10 $\mu$g without any significant reduction in the sensitivity. Operation under ambient conditions and a simple all-electrical design of the magnetometer should allow for an easy integration with other experimental setups. The uniaxial magnetic anisotropy of a 25 $\mu$m diameter iron wire, measured under ambient conditions with a high signal to noise ratio, was found to be in good agreement with its literature value. Further applications of the technique are discussed.
1404.6341v2
2014-05-02
Spectral line broadening in magnetized black holes
We consider weakly magnetized non-rotating black holes. In the presence of a regular magnetic field the motion of charged particles in the vicinity of a black hole is modified. As a result, the position of the innermost stable circular orbit (ISCO) becomes closer to the horizon. When the Lorentz force is repulsive (directed from the black hole) the ISCO radius can reach the gravitational radius. In the process of accretion charged particles (ions) of the accreting matter can be accumulated near their ISCO, while neutral particles fall down to the black hole after they reach $6M$ radius. The sharp spectral line Fe K$\alpha$, emitted by iron ions at such orbits, is broadened when the emission is registered by a distant observer. In this paper we study this broadening effect and discuss how one can extract information concerning the strength of the magnetic field from the observed spectrum.
1405.0510v3
2014-05-06
Evolution from incoherent to coherent electronic states and its implications to superconductivity in FeTe1-xSex
We have performed systematic angle-resolved photoemission spectroscopy (ARPES) of iron-chalcogenide superconductor FeTe1-xSex to elucidate the electronic states relevant to the superconductivity. While the Fermi-surface shape is nearly independent of x, we found that the ARPES spectral line shape shows prominent x dependence. A broad ARPES spectrum characterized by a small quasiparticle weight at x = 0, indicative of incoherent electronic states, becomes progressively sharper with increasing x, and a well-defined quasiparticle peak appears around x = 0.45 where bulk superconductivity is realized. The present result suggests the evolution from incoherent to coherent electronic states and its close relationship to the emergence of superconductivity.
1405.1172v1
2014-05-05
Mathematical Modeling on Open Limestone Channel
Acid mine drainage (AMD) is the outflow of acidic water from metal mines or coal mines. When exposed to air and water, metal sulfides from the deposits of the mines are oxidized and produce acid, metal ions and sulfate, which lower the pH value of the water. An open limestone channel (OLC) is a passive and low cost way to neutralize AMD. The dissolution of calcium into the water increases the pH value of the solution. A differential equation model is numerically solved to predict the variation of concentration of each species in the OLC solution. The diffusion of Calcium due to iron precipitates is modeled by a linear equation. The results give the variation of pH value and the concentration of Calcium.
1405.1338v1
2014-05-08
Effect of nominal substitution of transition metals for excess Fe in Fe_{1+x}Se superconductor
Taking cue from the increase in the superconducting transition temperature (Tc) of Fe1+xSe via nominal (2 wt%) substitution of Cr instead of excess Fe, we have now extended our study with nominal substitution (<=5 wt%) with other transition metals (Ni, Co, Fe, Mn, Cr, V and Ti) in place of excess iron. The Tc is found to increase (maximum ~11 K) or get suppressed depending on the substituted transition metal. Our studies indicate that the superconducting transition temperature depends on various parameters like the ionic size of the transition metal, its magnetic moment as well as the amount of hexagonal phase present as impurity.
1405.2050v3
2014-05-13
Magnetism and superconductivity in Sr$_2$VFeAsO$_3$ revealed by $^{75}$As- and $^{51}$V-NMR under elevated pressures
We report $^{75}$As- and $^{51}$V-nuclear magnetic resonance (NMR) measurements on the iron-based superconductor Sr$_2$VFeAsO$_3$ with alternating stacks structure. We find that the $^{75}$As nuclear spin-spin relaxation rate ($1/T_2$) shows a pronounced peak at $T_N$ = 165 K, below which the resonance peak shifts to a higher frequency due to the onset of an internal magnetic field. The $^{51}$V spectrum does not shift, but is broadened below $T_N$. We conclude that the Fe electrons oder antiferromagnetically below $T_N$ with a magnetic moment $m_{Fe}$ $\sim$ 0.4 $\mu_B$. Application of external pressure up to 2.4 GPa reduces $T_N$ in a rate of $-$40 K/GPa, and enhances the superconducting transition temperature $T_c$ in a rate of 2 K/GPa. The pressure-temperature phase diagram for Sr$_2$VFeAsO$_3$ shows that superconductivity coexists with antiferromagnetism over a wide pressure range with an unprecedented high $T_c$ up to 36.5 K.
1405.3048v1
2014-05-15
Nuclear Target Cross Section Ratios at MINERvA
Measurements of $\nu_{\mu}$ inclusive charged-current cross section ratios on carbon, iron, and lead relative to scintillator are presented. Data for the analysis were collected by the fine-grained MINERvA detector in the NuMI beamline at Fermilab. This is the first direct measurement of nuclear dependence in neutrino scattering. The ratios show a depletion at low Bjorken $x$ and enhancement at large $x$, both of which increase with the nucleon number of the target. The data exhibit trends not found in GENIE, a standard neutrino-nucleus event generator, or alternative models of nuclear modification to inelastic structure functions.
1405.3960v1
2014-05-19
Neutron Scattering Measurements of Spatially Anisotropic Magnetic Exchange Interactions in Semiconducting K0.85Fe1.54Se2 (TN=280 K)
We use neutron scattering to study the spin excitations associated with the stripe antiferromagnetic (AFM) order in semiconducting K$_{0.85}$Fe$_{1.54}$Se$_2$ ($T_N$=$280$ K). We show that the spin wave spectra can be accurately described by an effective Heisenberg Hamiltonian with highly anisotropic in-plane couplings at $T$= $5$ K. At high temperature ($T$= $300$ K) above $T_N$, short range magnetic correlation with anisotropic correlation lengths are observed. Our results suggest that, despite the dramatic difference in the Fermi surface topology, the in-plane anisotropic magnetic couplings are a fundamental property of the iron based compounds; this implies that their antiferromagnetism may originate from local strong correlation effects rather than weak coupling Fermi surface nesting.
1405.4737v1
2014-05-19
Multiferroic Iron Oxide Thin Films at Room-Temperature
In spite of being highly relevant for the development of a new generation of information storage devices, not many single-phase materials displaying magnetic and ferroelectric orders above room temperature are known. Moreover, these uncommon materials typically display insignificant values of the remanent moment in one of the ferroic orders or are complex multicomponent oxides which will be very challenging to integrate in devices. Here we report on the strategy to stabilize the metastable epsilon-Fe2O3 in thin film form, and we show that besides its already known ferrimagnetic nature, the films are also ferroelectric at 300 K with a remanent polarization of 1 microC/cm2. The film polarization shows long retention times and can be switched under small applied voltages. These characteristics make of epsilon-Fe2O3 the first single-ion transition-metal oxide which is ferro(ferri)magnetic and ferroelectric at room temperature. The simple composition of this new multiferroic oxide and the discovery of a robust path for its thin film growth may boost the exploitation of epsilon-Fe2O3 in novel devices.
1405.4909v1
2014-05-22
Layered water Cherenkov detector for the study of ultra high energy cosmic rays
We present a new design for the water Cherenkov detectors that are in use in various cosmic ray observatories. This novel design can provide a significant improvement in the independent measurement of the muonic and electromagnetic component of extensive air showers. From such multi-component data an event by event classification of the primary cosmic ray mass becomes possible. According to popular hadronic interaction models, such as EPOS-LHC or QGSJetII-04, the discriminating power between iron and hydrogen primaries reaches Fisher values of $\sim$ 2 or above for energies in excess of $10^{19}$ eV with a detector array layout similar to that of the Pierre Auger Observatory.
1405.5699v1
2014-05-25
Theory of Point Contact Spectroscopy in Correlated Materials
We develop a microscopic theory for the point-contact conductance between a metalic electrode and a strongly correlated material using the non-equilibrium Schwinger-Kadanoff-Baym-Keldysh formalism. We explicitly show that in the classical limit, contact size shorter than the scattering length of the system, the microscopic model can be reduced to an effective model with transfer matrix elements that conserve in-plane momentum. We find that the conductance $dI/dV$ is proportional to the {\it effective density of states}, that is, the integrated single-particle spectral function $A(\omega=eV)$ over the whole Brillouin zone. From this conclusion, we are able to establish the conditions under which a non-Fermi liquid metal exhibits a zero-bias peak in the conductance. This finding is discussed in the context of recent point-contact spectroscopy on the iron pnictides and chalcogenides which has exhibited a zero-bias conductance peak.
1405.6357v2
2014-05-25
CaFeAs$_2$: a Staggered Intercalation of Quantum Spin Hall and High Temperature Superconductivity
We predict that CaFeAs$_2$, a newly discovered iron-based high temperature (T$_c$) superconductor, is a staggered intercalation compound that integrates topological quantum spin hall (QSH) and superconductivity (SC). CaFeAs$_2$ has a structure with staggered CaAs and FeAs layers. While the FeAs layers are known to be responsible for high T$_c$ superconductivity, we show that with spin orbital coupling each CaAs layer is a $Z_{2}$ topologically nontrivial two-dimensional QSH insulator and the bulk is a 3-dimensional weak topological insulator. In the superconducting state, the edge states in the CaAs layer are natural 1D topological superconductors. The staggered intercalation of QSH and SC provides us an unique opportunity to realize and explore novel physics, such as Majorana modes and Majorana Fermions chains.
1405.6401v2
2014-05-28
Contactless measurement of nonlinear conductivity in the radio-frequency range
We have developed a system for contactless measurement of nonlinear conductivity in the radio-frequency band, and over a wide temperature range. A non-resonant circuit is used to electrically excite the sample, and the induced signal is detected by a resonant circuit whose natural frequency matches higher harmonics of the excitation. A simple modification of the probe allows non-resonant detection suitable for stronger signals. Two measurement procedures are proposed that allow significant excitation power variation, up to 150 W. The apparatus has been validated trough the measurement of the nonlinear response at the superconducting transition of a high-Tc superconductor, and the nematic transition of an iron pnictide.
1405.7282v1
2014-05-31
Point contact spectroscopy in the superconducting and normal state of $\mathrm{NaFe_{1-\textit{x}}Co_\textit{x}As}$
We use point contact spectroscopy to probe the superconducting and normal state properties of the iron-based superconductor $\rm{NaFe_{1-\textit{x}}Co_{\textit{x}}As}$ with $\rm{\textit{x} = 0, 0.02, 0.06}$. Andreev spectra corresponding to multiple superconducting gaps are detected in the superconducting phase. For $\rm{\textit{x} = 0.02}$, a broad conductance enhancement around zero bias voltage is detected in both the normal and the superconducting phase. Such a feature is not present in the $\rm{\textit{x} = 0.06}$ samples. We suspect that this enhancement is caused by orbital fluctuations, as previously detected in underdoped $\rm{Ba(Fe_{1-\textit{x}}Co_\textit{x})_2As_2}$ (Phys. Rev. B 85, 214515 (2012)). Occasionally, the superconducting phase shows a distinct asymmetric conductance feature instead of Andreev reflection. We discuss the possible origins of this feature. NaFeAs (the parent compound) grown by two different techniques is probed. Melt-grown NaFeAs shows a normal state conductance enhancement. On the other hand, at low temperatures, flux-grown NaFeAs shows a sharp dip in the conductance at zero bias voltage. The compounds are very reactive in air and the different spectra are likely a reflection of their different oxidation and purity levels.
1406.0038v1
2014-06-01
Hydrogen-Activation Mechanism of [Fe] Hydrogenase Revealed by Multi-Scale Modeling
When investigating the mode of hydrogen activation by [Fe] hydrogenases, not only the chemical reactivity at the active site is of importance but also the large-scale conformational change between the so-called open and closed conformations, which leads to a special spatial arrangement of substrate and iron cofactor. To study H2 activation, a complete model of the solvated and cofactor-bound enzyme in complex with the substrate methenyl-H4MPT+ was constructed. Both the closed and open conformations were simulated with classical molecular dynamics on the 100 ns time scale. Quantum-mechanics/molecular-mechanics calculations on snapshots then revealed the features of the active site that enable the facile H2 cleavage. The hydroxyl group of the pyridinol ligand can easily be deprotonated. With the deprotonated hydroxyl group and the structural arrangement in the closed conformation, H2 coordinated to the Fe center is subject to an ionic and orbital push-pull effect and can be rapidly cleaved with a concerted hydride transfer to methenyl-H4MPT+. An intermediary hydride species is not formed.
1406.0166v1
2014-06-04
Observation of strong electron pairing on bands without Fermi surfaces in LiFe1-xCoxAs
In conventional BCS superconductors, the quantum condensation of superconducting electron pairs is understood as a Fermi surface (FS) instability, in which the low-energy electrons are paired by attractive interactions. Whether this explanation is still valid in high-Tc superconductors such as cuprates and iron-based superconductors remains an open question. In particular, a fundamentally different picture of the electron pairs, which are believed to be formed locally by repulsive interactions, may prevail. Here we report a high-resolution angle-resolved photoemission spectroscopy study on LiFe1-xCoxAs. We reveal a large and robust superconducting (SC) gap on a band sinking below the Fermi energy upon Co substitution. The observed FS-free SC order is also the largest over the momentum space, which rules out a proximity effect origin and indicates that the SC order parameter is not tied to the FS as a result of a FS instability.
1406.0983v2
2014-06-04
Anomalous Nernst and Hall effects in magnetized platinum and palladium
We study the anomalous Nernst effect (ANE) and anomalous Hall effect (AHE) in proximity-induced ferromagnetic palladium and platinum which is widely used in spintronics, within the Berry phase formalism based on the relativistic band structure calculations. We find that both the anomalous Hall ($\sigma_{xy}^A$) and Nernst ($\alpha_{xy}^A$) conductivities can be related to the spin Hall conductivity ($\sigma_{xy}^S$) and band exchange-splitting ($\Delta_{ex}$) by relations $\sigma_{xy}^A =\Delta_{ex}\frac{e}{\hbar}\sigma_{xy}^S(E_F)'$ and $\alpha_{xy}^A = -\frac{\pi^2}{3}\frac{k_B^2T\Delta_{ex}}{\hbar}\sigma_{xy}^s(\mu)"$, respectively. In particular, these relations would predict that the $\sigma_{xy}^A$ in the magnetized Pt (Pd) would be positive (negative) since the $\sigma_{xy}^S(E_F)'$ is positive (negative). Furthermore, both $\sigma_{xy}^A$ and $\alpha_{xy}^A$ are approximately proportional to the induced spin magnetic moment ($m_s$) because the $\Delta_{ex}$ is a linear function of $m_s$. Using the reported $m_s$ in the magnetized Pt and Pd, we predict that the intrinsic anomalous Nernst conductivity (ANC) in the magnetic platinum and palladium would be gigantic, being up to ten times larger than, e.g., iron, while the intrinsic anomalous Hall conductivity (AHC) would also be significant.
1406.1029v1
2014-06-09
Magnetic and orbital instabilities in a lattice of SU(4) organometallic Kondo complexes
Motivated by experiments of scanning tunneling spectroscopy (STS) on self-assembled networks of iron(II)-phtalocyanine (FePc) molecules deposited on a clean Au(111) surface [FePc/Au(111)] and its explanation in terms of the extension of the impurity SU(4) Anderson model to the lattice in the Kondo regime, we study the competition between the Kondo effect and the magneto-orbital interactions occurring in FePc/Au(111). We explore the quantum phases and critical points of the model using a large-$N$ slave-boson method in the mean-field approximation. The SU(4) symmetry in the impurity appears as a combination of the usual spin and an orbital pseudospin arising from the degenerate $3d_{xz}$ and $3d_{yz}$ orbitals in the Fe atom. In the case of the lattice, our results show that the additional orbital degrees of freedom crucially modify the low-temperature phase diagram, and induce new types of orbital interactions among the Fe atoms, which can potentially stabilize exotic quantum phases with magnetic and orbital order. The dominant instability corresponds to spin ferromagnetic and orbital antiferromagnetic order.
1406.2347v1
2014-06-11
ARPES experiment in fermiology of quasi-2D metals (Review Article)
Angle resolved photoemission spectroscopy (ARPES) enables direct observation of the Fermi surface and underlying electronic structure of crystals---the basic concepts to describe all the electronic properties of solids and to understand the key electronic interactions involved. The method is the most effective to study quasi-2D metals, to which the subjects of almost all hot problems in modern condensed matter physics have happened to belong. This has forced incredibly the development of the ARPES method which we face now. The aim of this paper is to introduce to the reader the state-of-the-art ARPES, reviewing the results of its application to such topical problems as high temperature superconductivity in cuprates and iron based superconductors, and electronic ordering in the transition metal dichalcogenides and manganites.
1406.2948v1
2014-06-14
Critical Behavior of the SDW Transition in Underdoped Ba(Fe1-xCox)2As2 (x <=0.05): 75As NMR Investigation
We investigate the nature of the SDW (Spin Density Wave) transition in the underdoped regime of an iron-based high Tc superconductor Ba(Fe1-xCox)2As2 by 75As NMR, with primary focus on a composition with x = 0.02 (T_SDW = 99 K).We demonstrate that critical slowing down toward the three dimensional SDW transition sets in at the tetragonal to orthorhombic structural phase transition, Ts = 105 K, suggesting strong interplay between structural distortion and spin correlations. In the critical regime between Ts and T_SDW, the dynamical structure factor of electron spins S(q,Wn) measured with the longitudinal NMR relaxation rate 1/T1 exhibits a divergent behavior obeying a power law, 1/T1~S(q, Wn)~(T/T_SDW-1)^a with the critical exponent a ~ 0.33.
1406.3734v1
2014-06-16
Search for Magnetic Monopole using ICAL at INO
Sub-relativistic magnetic monopoles are predicted from the GUT era by theory. To date there have been no confirmed observations of such exotic particles. The Iron CALorimeter (ICAL) at India-based Neutrino Observatory (INO) aims to measure the neutrino oscillation parameters precisely. As it is a tracking detector there is also the possibility of detecting magnetic monopoles in the sub-relativistic region. Using ICAL the magnetic monopole event is characterised by the large time intervals of upto 30 microsec between the signals in successive layers of the active detectors. The aim of this study is to identify the sensitivity of ICAL for a particle carrying magnetic charge in the mass range from 10^{5} to 10^{17} GeV with beta ranging from 10^{-5} to 9 x 10^{-1} for ICAL at INO. A similar study has also been carried out for the ICAL prototype which will be placed overground. Due to the rock cover of approximately 1.3 km, ICAL at INO will not be able to place bounds on the flux of the lower mass magnetic monopoles. This mass region is however addressed by the prototype ICAL.
1406.3938v1
2014-06-16
An air-cooled Litz wire coil for measuring the high frequency hysteresis loops of magnetic samples : a useful setup for magnetic hyperthermia applications
A low-cost and simple setup for measuring the high-frequency hysteresis loops of magnetic samples is described. An AMF in the range 6-100 kHz with amplitude up to 80 mT is produced by a Litz wire coil. The latter is air-cooled using a forced-air approach so no water flow is required to run the setup. High-frequency hysteresis loops are measured using a system of pick-up coils and numerical integration of signals. Reproducible measurements are obtained in the frequency range of 6-56 kHz. Measurement examples on ferrite cylinders and on iron oxide nanoparticle ferrofluids are shown. Comparison with other measurement methods of the hysteresis loop area (complex susceptibility, quasi-static hysteresis loops and calorific measurements) is provided and shows the coherency of the results obtained with this setup. This setup is well adapted to the magnetic characterization of colloidal solutions of MNPs for magnetic hyperthermia applications.
1406.4013v1
2014-06-16
Infrared dichroism of gold nanorods controlled using a magnetically addressable mesophase
Gold nanorods have unique optical properties, which make them promising candidates for building nano-structured materials using a "bottom-up" strategy. We formulate stable bulk materials with anisotropic optical properties by inserting gold and iron oxide nanorods within a lamellar mesophase. Quantitative measurements of the order parameter by modelling the absorbance spectra show that the medium is macroscopically aligned in a direction defined by an external magnetic field. Under field, the system exhibits significant absorption dichroism in the infrared range, at the position of the longitudinal plasmon peak of the gold nanorods (about 1200 nm), indicating strong confinement of these particles within the water layers of the lamellar phase. This approach can yield soft and addressable optical elements.
1406.4014v1
2014-06-21
The Deaths of Very Massive Stars
The theory underlying the evolution and death of stars heavier than 10 Msun on the main sequence is reviewed with an emphasis upon stars much heavier than 30 Msun. These are stars that, in the absence of substantial mass loss, are expected to either produce black holes when they die, or, for helium cores heavier than about 35 Msun, encounter the pair instability. A wide variety of outcomes is possible depending upon the initial composition of the star, its rotation rate, and the physics used to model its evolution. These heavier stars can produce some of the brightest supernovae in the universe, but also some of the faintest. They can make gamma-ray bursts or collapse without a whimper. Their nucleosynthesis can range from just CNO to a broad range of elements up to the iron group. Though rare nowadays, they probably played a disproportionate role in shaping the evolution of the universe following the formation of its first stars.
1406.5657v1
2014-06-22
Variation of the X-ray non-thermal emission in the Arches cloud
The origin of the iron fluorescent line at 6.4 keV from an extended region surrounding the Arches cluster is debated and the non-variability of this emission up to 2009 has favored the low-energy cosmic-ray origin over a possible irradiation by hard X-rays. By probing the variability of the Arches cloud non-thermal emission in the most recent years, including a deep observation in 2012, we intend to discriminate between the two competing scenarios. We perform a spectral fit of XMM-Newton observations collected from 2000 to 2013 in order to build the Arches cloud lightcurve corresponding to both the neutral Fe Kalpha line and the X-ray continuum emissions. We reveal a 30% flux drop in 2012, detected with more than 4 sigma significance for both components. This implies that a large fraction of the studied non-thermal emission is due to the reflection of an X-ray transient source.
1406.5727v1
2014-06-22
Putnam looks at quantum mechanics (again and again)
Hilary Putnam (1965, 2005) has argued that from a realist perspective, quantum mechanics stands in need of an interpretation. Ironically, this hypothesis may appear vulnerable against arguments drawing on Putnam's own work. Nancy Cartwright (2005) has urged that his 1962 essay on the meaning of theoretical terms suggests that quantum mechanics needs no interpretation and thus stands in tension with his claim of three years later. She furthermore contends that this conflict should be resolved in favour of the earlier work, as quantum mechanics, like all successful theories, does not need an interpretation. The first part of this essay deflates both of these objections. The second part addresses and evaluates Putnam's own assessments of the main interpretative options available in 1965 and 2005. Although we may disagree on some aspects, his pessimistic conclusion will come out largely unscathed, and, in fact, enhanced. I will close by briefly stating the historical relevance of this work.
1406.5737v1
2014-06-23
Phonon Anomalies, Orbital-Ordering and Electronic Raman Scattering in iron-pnictide Ca(Fe0.97Co0.03)2As2: Temperature-dependent Raman Study
We report inelastic light scattering studies on Ca(Fe0.97Co0.03)2As2 in a wide spectral range of 120-5200 cm-1 from 5K to 300K, covering the tetragonal to orthorhombic structural transition as well as magnetic transition at Tsm ~ 160K. The mode frequencies of two first-order Raman modes B1g and Eg, both involving displacement of Fe atoms, show sharp increase below Tsm. Concomitantly, the linewidths of all the first-order Raman modes show anomalous broadening below Tsm, attributed to strong spin-phonon coupling. The high frequency modes observed between 400-1200 cm-1 are attributed to the electronic Raman scattering involving the crystal field levels of d-orbitals of Fe2+. The splitting between xz and yz d-orbital levels is shown to be ~ 25 meV which increases as temperature decreases below Tsm. A broad Raman band observed at ~ 3200 cm-1 is assigned to two-magnon excitation of the itinerant Fe 3d antiferromagnet.
1406.5844v1
2014-06-30
Interplay of magnetism and superconductivity in EuFe$_{2}$(As$_{1-x}$P$_{x}$)$_{2}$ single crystals probed by muon spin rotation and ${}^{57}$Fe Mössbauer spectroscopy
We present our results of a local probe study on EuFe$_{2}$(As$_{1-x}$P$_{x}$)$_{2}$ single crystals with $x$=0.13, 0.19 and 0.28 by means of muon spin rotation and ${}^{57}$Fe M\"ossbauer spectroscopy. We focus our discussion on the sample with $x$=0.19 viz. at the optimal substitution level, where bulk superconductivity ($T_{\text{SC}}=28$ K) sets in above static europium order ($T^{\text{Eu}}=20$K) but well below the onset of the iron antiferromagnetic (AFM) transition ($\sim$100 K). We find enhanced spin dynamics in the Fe sublattice closely above $T_{\text{SC}}$ and propose that these are related to enhanced Eu fluctuations due to the evident coupling of both sublattices observed in our experiments.
1406.7715v1
2014-06-30
Theoretical Analysis of Bayesian Optimisation with Unknown Gaussian Process Hyper-Parameters
Bayesian optimisation has gained great popularity as a tool for optimising the parameters of machine learning algorithms and models. Somewhat ironically, setting up the hyper-parameters of Bayesian optimisation methods is notoriously hard. While reasonable practical solutions have been advanced, they can often fail to find the best optima. Surprisingly, there is little theoretical analysis of this crucial problem in the literature. To address this, we derive a cumulative regret bound for Bayesian optimisation with Gaussian processes and unknown kernel hyper-parameters in the stochastic setting. The bound, which applies to the expected improvement acquisition function and sub-Gaussian observation noise, provides us with guidelines on how to design hyper-parameter estimation methods. A simple simulation demonstrates the importance of following these guidelines.
1406.7758v1
2014-07-01
Emergent defect states as a source of resistivity anisotropy in the nematic phase of iron pnictides
We consider the role of potential scatterers in the nematic phase of Fe-based superconductors above the transition temperature to the (pi,0) magnetic state but below the orthorhombic structural transition. The anisotropic spin fluctuations in this region can be frozen by disorder, to create elongated magnetic droplets whose anisotropy grows as the magnetic transition is approached. Such states act as strong anisotropic defect potentials which scatter with much higher probability perpendicular to their length than parallel, although the actual crystal symmetry breaking is tiny. We calculate the scattering potentials, relaxation rates, and conductivity in this region, and show that such emergent defect states are essential for the transport anisotropy observed in experiments.
1407.0117v1
2014-07-01
Anomalous ideal tensile strength of ferromagnetic Fe and Fe-rich alloys
Within the same failure mode, iron has the lowest ideal tensile strength among the transition metals crystallizing in the body-centered cubic structure. Here, we demonstrate that this anomalously low strength of Fe originates partly from magnetism and is reflected in unexpected alloying effects in dilute Fe(\emph{M}) (\emph{M} = Al, V, Cr, Mn, Co, Ni) binaries. We employ the structural energy difference and the magnetic pressure to disentangle the magnetic effect on the ideal tensile strength from the chemical effect. We find that the investigated solutes strongly alter the magnetic response of the Fe host from the weak towards a stronger ferromagnetic behavior, which is explained based on single-particle band energies.
1407.0289v1
2014-07-03
The electronic structure of Co-substituted $\textrm{Fe}\textrm{Se}$ superconductor probed by soft X-ray spectroscopy and density functional theory
We study the crystalline and electronic properties of the $\textrm{Fe}_{1-x}\textrm{Co}_x\textrm{Se}$ system ($x=0$, 0.25, 0.5, 0.75, and 1.0) using X-ray diffraction, X-ray spectroscopy and density functional theory. We show that the introduction of Co $3d$ states in FeSe relaxes the bond strengths and induces a structural transition from tetragonal to hexagonal whose crossover takes place at $x\approx0.38$. This structural transition in turn modifies the magnetic order which can be related to the spin state. Using resonant inelastic X-ray spectroscopy we estimate the spin state of the system; FeSe is found to be in a high spin state (S=2), but Fe is reduced to a low spin state upon Co substitution of $x \le 0.25$, well below the structural transition. Finally, we show evidence that FeSe is a moderately correlated system but the introduction of Co into the host lattice weakens the correlation strength for $x\ge0.25$. These novel findings are important to unravel the mechanisms responsible for the superconducting state in iron-chalcogenide superconductors.
1407.0746v1
2014-07-03
A Tale of Three Galaxies: Anomalous Dust Properties in IRASF10398+1455, IRASF21013-0739 and SDSSJ0808+3948
On a galactic scale the 9.7um silicate emission is usually only seen in type 1 active galactic nuclei (AGNs). They usually also display a flat emission continuum at ~5--8um and the absence of polycyclic aromatic hydrocarbon (PAH) emission bands. In contrast, starburst galaxies, luminous infrared (IR) galaxies (LIRGs), and ultraluminous IR galaxies (ULIRGs) exhibit a red 5--8um emission continuum, strong 10um and 18um silicate absorption features, and strong PAH emission bands. Here we report the detection of anomalous dust properties by Spitzer/Infrared Spectrograph in three galaxies (IRASF10398+1455, IRASF21013-0739 and SDSSJ0808+3948) which are characterized by the simultaneous detection of a red 5--8um emission continuum, the 9.7 and 18um silicate emission features as well as strong PAH emission bands. These apparently contradictory dust IR emission properties are discussed in terms of iron-poor silicate composition, carbon dust deficit, small grain size and low dust temperature in the young AGN phase of these three galaxies.
1407.0914v3
2014-07-03
Superconductivity by rare earth doping in the 1038-type compounds (Ca$_{1-x}$RE$_x$)$_{10}$(FeAs)$_{10}$(Pt$_3$As$_8$) with RE = Y, La-Nd, Sm-Lu
We report superconductivity in polycrystalline samples of the 1038-type compounds (Ca$_{1-x}$RE$_x$)$_{10}$(FeAs)$_{10}$(Pt$_3$As$_8$) up to T$_c$ = 35 K with RE = Y, La-Nd, Sm, Gd-Lu. The critical temperatures are independent of the trivalent rare earth element used, yielding an universal T$_c$($x$) phase diagram for electron doping in all these systems. The absence of superconductivity in Eu$^{2+}$ doped samples, as well as the close resemblance of (Ca$_{1-x}$RE$_x$)$_{10}$(FeAs)$_{10}$(Pt$_3$As$_8$) to the 1048 compound substantiate that the electron doping scenario in the RE-1038 and 1048 phases is completely analogous to other iron-based superconductors with simpler crystal structures.
1407.1007v1
2014-07-05
Self-organized electronic superlattices in layered materials
We show that in layered systems with electronic phase separation tendency, the long-range Coulomb interaction can drive the spontaneous formation of unidirectional superlattices of electronic charge in a completely homogeneous crystalline background. In this self-organized electronic heterostructure, the ratio among the number of crystalline planes in the minority and majority electronic phases corresponds to Farey fractions with the superlattice period controlled by the background charge density and the frustrating Coulomb interaction strength. The phase diagram displays Arnold tongues obeying a modified Farey tree hierarchy and a devil's staircase typical of systems with frustration among different scales. We further discuss the competition of these electronic superlattices, recently observed in iron-based superconductors and mixed valence compounds, with in-plane electronically modulated phases.
1407.1378v1
2014-07-10
NMR investigation of spin correlations in BaCo2As2
We use NMR techniques to investigate the magnetic properties of BaCo2As2 single crystals, the non-superconducting end member of the Co-substituted iron-pnictide high Tc superconductor Ba(Fe1-xCox)2As2 with x = 1. We present 75As NMR evidence for enhancement of low frequency spin fluctuations below ~ 100 K. This enhancement is accompanied by that of static uniform spin susceptibility at the wave vector q = 0, suggesting that the primary channel of the spin correlations is ferromagnetic rather than antiferromagnetic. Comparison between the NMR Knight shift 75K and bulk susceptibility chi(bulk) data uncovers the presence of two separate components of spin susceptibility with distinct temperature dependences, presumably because multiple electronic bands crossing the Fermi energy play different roles in the electronic properties of BaCo2As2.
1407.2750v1
2014-07-13
Accurate bare susceptibilities from full-potential $\textit{ab initio}$ calculations
Electronic susceptibilities are a very popular tool to study electronic and magnetic properties of materials, both in experiment and theory. Unfortunately, the numerical evaluation of even the bare susceptibility, which depends on the computation of matrix elements and sums over energy bands, is very work-intensive and therefore various approximations have been introduced to speed up the calculations. We present a reliable and efficient implementation to compute static as well as dynamic bare susceptibilities based on full-potential density functional theory (DFT) calculations. Based on the exact results we will assess the accuracy of replacing the matrix elements with a constant and the impact of truncating the sum over the energy bands. Results will be given for representative and topical materials, such as Cr, a classical transition metal, as well as for FeSe and LaFeAsO, examples of iron-based superconductors.
1407.3444v2
2014-07-14
Observation of pseudogap-like feature above Tc in LiFeAs and (Ba0.6K0.4)Fe2As2 by ultrafast optical measurement
We utilize ultrafast optical measurement to study the quasiparticle relaxation in stoichiometric LiFeAs and nearly optimally doped (BaK)Fe2As2 crystals. According to our temperature-dependent studies of LiFeAs, we have observed pseudogap-like feature at onset temperature of ~ 55 K, which is above Tc = 15 K. In addition, the onset temperature of pseudogap ~90K was also observed in Ba0.6K0.4Fe2As2 (Tc = 36 K). Our findings seem implying that the pseudogap feature, which is due to antiferromagnetic fluctuations, is universal for the largely studied 11, 111, 122, and 1111 iron-based superconductors.
1407.3539v1
2014-07-16
The Effect of Doppler Broadening on the $6.3 \ PeV$ $W^-$ Resonance in $\barν_e e^-$ Collisions
We calculate the Doppler broadening of the $W^-$ resonance produced in $\bar{\nu}_e e^-$ collisions of cosmic anti-neutrinos with $E_{\nu}\approx 6.3 \ PeV$ with electrons in atoms up to Iron. Revisiting this issue is prompted by recent observations of PeV neutrinos by Ice-Cube. Despite its poor energy resolution, the $20\%$ Doppler broadening of the resonance due to electronic motions can produce observable effects via non-linear neutrino absorption near the resonance. The attendant suppression of the peak cross section allows $\bar{\nu}_e$ to travel correspondingly longer distances. While this effect is unlikely to be directly detected in the near future, it may facilitate terrestrial tomography at depths of $\sim 10 \ km$, complementing deeper explorations using the more frequent nuclear interactions at lower energies.
1407.4415v1
2014-07-17
Spatial ordering of nano-dislocation loops in ion-irradiated materials
Defect microstructures formed in ion-irradiated metals, for example iron or tungsten, often exhibit patterns of spatially ordered nano-scale dislocation loops. We show that such ordered dislocation loop structures may form spontaneously as a result of Brownian motion of loops, biased by the angular-dependent elastic interaction between the loops. Patterns of spatially ordered loops form once the local density of loops produced by ion irradiation exceeds a critical threshold value.
1407.4683v1
2014-07-18
Estimating R-Process Yields from Abundances of the Metal-Poor Stars
The chemical abundances of metal-poor stars provide important clues to explore stellar formation history and set significant constraints on models of the r-process. In this work, we find that the abundance patterns of the light and iron group elements of the main r-process stars are very close to those of the weak r-process stars. Based on a detailed abundance comparison, we find that the weak r-process occurs in supernovae with a progenitor mass range of $\sim11-26M_{\odot}$. Using the SN yields given by Heger & Woosley and the abundances of the weak r-process stars, the weak r-process yields are derived. The SNe with a progenitor mass range of $15M_{\odot}<M<26M_{\odot}$ are the main sites of the weak r-process and their contributions are larger than 80%. Using the abundance ratios of the weak r-process and the main r-process in the solar system, the average yields of the main r-process are estimated. The observed correlations of the [neutron-capture/Eu] versus [Eu/Fe] can be explained by mixing of the two r-process abundances in various fractions.
1407.4878v1
2014-07-22
Orbital Selective Mott Transition Induced by Orbitals with Distinct Noninteracting Densities of States
By applying dynamical mean-field theory in combination with exact diagonalization at zero temperature to a half-filled Hubbard model with two orbitals having distinct noninteracting densities of states, we show that an orbital selective Mott transition (OSMT) will take place even without crystal field splitting, differences in bandwidth and orbital degeneracy. We find that formation of local spin triplet states followed by a two-stage breakdown of the Kondo effect, rather than decoupling of charge degrees of freedom among different orbitals, is the underlying physics for the OSMT. The relevance of our findings to Ca$_{2-x}$Sr$_x$RuO$_4$ and the iron-based superconductors is discussed, and a decent candidate to detect such an origin for the OSMT is proposed.
1407.5795v1
2014-07-31
Improving the Scalability of DPWS-Based Networked Infrastructures
The Devices Profile for Web Services (DPWS) specification enables seamless discovery, configuration, and interoperability of networked devices in various settings, ranging from home automation and multimedia to manufacturing equipment and data centers. Unfortunately, the sheer simplicity of event notification mechanisms that makes it fit for resource-constrained devices, makes it hard to scale to large infrastructures with more stringent dependability requirements, ironically, where self-configuration would be most useful. In this report, we address this challenge with a proposal to integrate gossip-based dissemination in DPWS, thus maintaining compatibility with original assumptions of the specification, and avoiding a centralized configuration server or custom black-box middleware components. In detail, we show how our approach provides an evolutionary and non-intrusive solution to the scalability limitations of DPWS and experimentally evaluate it with an implementation based on the the Web Services for Devices (WS4D) Java Multi Edition DPWS Stack (JMEDS).
1407.8546v1